TY - JOUR
T1 - Ozone-activated lignocellulose films blended with chitosan for edible film production
AU - Ebrahimi, Seyedeh Sedigheh
AU - Hamzeh, Yahya
AU - Ashori, Alireza
AU - Roohani, Mehdi
AU - Marlin, Nathalie
AU - Spigno, Giorgia
PY - 2024
Y1 - 2024
N2 - This work focuses on the influence of ozone pretreatment on the fractionation and solubilization of sugarcane bagasse and soda bagasse pulp fibers in sodium hydroxide/urea solution, as well as the application of regenerated cellulose for producing edible films. The methodology involved pretreating lignocelluloses with ozone for 20 to 120 min before dissolving in sodium hydroxide/urea solution. The influence of the pretreatment conditions on cellulose dissolution yield was investigated. Regenerated cellulose films were then formed, with and without the addition of 2 % chitosan. Mechanical, physical, structural, thermal, and antimicrobial attributes were determined as a function of ozonation conditions of raw materials and chitosan content. The findings exhibited positive effects of short ozonation on enhancing mechanical strength, cohesion, and hydrophobicity. The prolonged ozonation of 120 min demonstrated optimal improvements in continuity, swelling, and antibacterial resistance of obtained films. Incorporating chitosan enhanced tensile performance, stiffness, and vapor barriers but increased moisture absorption. Tailoring the activation of biomass through ozone pretreatment and chitosan addition resulted in renewable films with adjustable properties to meet diverse packaging requirements, particularly for fruit protective coatings, ensuring the preservation of post-harvest quality.
AB - This work focuses on the influence of ozone pretreatment on the fractionation and solubilization of sugarcane bagasse and soda bagasse pulp fibers in sodium hydroxide/urea solution, as well as the application of regenerated cellulose for producing edible films. The methodology involved pretreating lignocelluloses with ozone for 20 to 120 min before dissolving in sodium hydroxide/urea solution. The influence of the pretreatment conditions on cellulose dissolution yield was investigated. Regenerated cellulose films were then formed, with and without the addition of 2 % chitosan. Mechanical, physical, structural, thermal, and antimicrobial attributes were determined as a function of ozonation conditions of raw materials and chitosan content. The findings exhibited positive effects of short ozonation on enhancing mechanical strength, cohesion, and hydrophobicity. The prolonged ozonation of 120 min demonstrated optimal improvements in continuity, swelling, and antibacterial resistance of obtained films. Incorporating chitosan enhanced tensile performance, stiffness, and vapor barriers but increased moisture absorption. Tailoring the activation of biomass through ozone pretreatment and chitosan addition resulted in renewable films with adjustable properties to meet diverse packaging requirements, particularly for fruit protective coatings, ensuring the preservation of post-harvest quality.
KW - Bagasse fibers
KW - Chitosan
KW - Ozone pretreatment
KW - Lignocellulose films
KW - Edible film
KW - Bagasse fibers
KW - Chitosan
KW - Ozone pretreatment
KW - Lignocellulose films
KW - Edible film
UR - http://hdl.handle.net/10807/288376
U2 - 10.1016/j.ijbiomac.2024.132285
DO - 10.1016/j.ijbiomac.2024.132285
M3 - Article
SN - 0141-8130
VL - 270
SP - N/A-N/A
JO - International Journal of Biological Macromolecules
JF - International Journal of Biological Macromolecules
ER -