TY - JOUR
T1 - Electric-field assisted optimal quantum transport of photo-excitations in polar heterostructures
AU - Kropf, Chahan M.
AU - Celardo, Giuseppe Luca
AU - Giannetti, Claudio
AU - Borgonovi, Fausto
PY - 2020
Y1 - 2020
N2 - Transition-metal-oxide (TMO) heterostructures are promising candidates for building photon-harvesting devices which can exploit optimal quantum transport of charge excitations generated by light absorption. Here we address the explicit role of an electric field on the quantum transport properties of photo-excitations subject to dephasing in one-dimensional chains coupled to a continuum of states acting as a sink. We show that the average transfer time to the sink is optimized for suitable values of both the coupling strength to the sink and the electric field, thus fully exploiting the coherence-enhanced efficiency in the quantum transport regime achievable in few monolayers TMO heterostructures. The optimal coupling to the continuum remains approximately the same as that in absence of electric field and is characterizing the Superradiant Transition. On the other hand, the optimal electric field for which we provide estimates using an analytical expression is dependent on the initial state.
AB - Transition-metal-oxide (TMO) heterostructures are promising candidates for building photon-harvesting devices which can exploit optimal quantum transport of charge excitations generated by light absorption. Here we address the explicit role of an electric field on the quantum transport properties of photo-excitations subject to dephasing in one-dimensional chains coupled to a continuum of states acting as a sink. We show that the average transfer time to the sink is optimized for suitable values of both the coupling strength to the sink and the electric field, thus fully exploiting the coherence-enhanced efficiency in the quantum transport regime achievable in few monolayers TMO heterostructures. The optimal coupling to the continuum remains approximately the same as that in absence of electric field and is characterizing the Superradiant Transition. On the other hand, the optimal electric field for which we provide estimates using an analytical expression is dependent on the initial state.
KW - Electric potential
KW - Open quantum systems
KW - Optimal quantum transport
KW - Quantum master equation
KW - Superradiance
KW - Transition-metal-oxide heterostructures
KW - Electric potential
KW - Open quantum systems
KW - Optimal quantum transport
KW - Quantum master equation
KW - Superradiance
KW - Transition-metal-oxide heterostructures
UR - http://hdl.handle.net/10807/152181
UR - https://www.sciencedirect.com/science/article/pii/s1386947719316017
U2 - 10.1016/j.physe.2020.114023
DO - 10.1016/j.physe.2020.114023
M3 - Article
SN - 1386-9477
VL - 120
SP - 114023
EP - 114033
JO - PHYSICA E-LOW-DIMENSIONAL SYSTEMS & NANOSTRUCTURES
JF - PHYSICA E-LOW-DIMENSIONAL SYSTEMS & NANOSTRUCTURES
ER -